Sayan_et_al-2018-International_Journal_of_Applied_Ceramic_Technology.pdf (1.96 MB)
Single-step fabrication of an anode supported planar single-chamber solid oxide fuel cell
journal contribution
posted on 2018-06-05, 12:12 authored by Yunus Sayan, Vijay Venkatesan, Erdogan Guk, Houzheng Wu, Jung-Sik KimWe present single-step-co-sintering manufacture of a planar single-chamber solid oxide fuel cell (SC-SOFC) with porous multilayer structures consisting of NiO/CGO, CGO and CGO-LSCF as anode, electrolyte, and cathode, respectively. Their green tapes were casted with 20 μm thickness and stacked into layers of anode, electrolyte, and cathode (10:2:2), then hot-pressed at 2 MPa and 60°C for 5 minutes (deemed optimal). Subsequently, hot laminated layers were cut into 40 × 40 mm cells and co-sintered up to 1200°C via different sintering profiles. Shrinkage behavior and curvature developments of cells were characterized, determining the best sintering profile. Hence, anode-supported SC-SOFCs were fabricated via a single-step co-sintering process, albeit with curvature formation at edges. Subsequently, anode thickness was increased to 800 μm and electrolyte reduced to 20 μm to obtain SOFCs with drastically reduced curvature with the help of a porous alumina cover plate.
Funding
The authors appreciate the support provided by the Turkish Ministry of Higher Education and partial financial support from the India-UK Collaborative Research Initiative in Fuel Cells project on “Modelling Accelerated Ageing and Degradation of Solid Oxide Fuel Cells (EP/I037059/1), and also the EPSRC’s UK-Korea Collaborative Research Activity in Fuel Cells project on “Novel diagnostic tools and techniques for monitoring and control of SOFC stacks” (EP/M02346X/1).
History
School
- Aeronautical, Automotive, Chemical and Materials Engineering
Department
- Materials
Published in
International Journal of Applied Ceramic TechnologyCitation
SAYAN, Y. ... et al, 2018. Single-step fabrication of an anode supported planar single-chamber solid oxide fuel cell. International Journal of Applied Ceramic Technology, 15(6), pp. 1375-138.Publisher
© The Authors.International Journal of Applied Ceramic Technology published by Wiley Periodicals, Inc. on behalf of American Ceramics SocietyVersion
- VoR (Version of Record)
Publisher statement
This work is made available according to the conditions of the Creative Commons Attribution 4.0 International (CC BY 4.0) licence. Full details of this licence are available at: http://creativecommons.org/licenses/by/4.0/Publication date
2018Notes
This work is made available according to the conditions of the Creative Commons Attribution 4.0 International (CC BY 4.0) licence. Full details of this licence are available at: http://creativecommons.org/licenses/by/4.0/ISSN
1546-542XeISSN
1744-7402Publisher version
Language
- en